A peer-reviewed journal published by K. N. Toosi University of Technology

Document Type : Research Article

Authors

1 Radiation Application Research School, Nuclear Science and Technology Research Institute, Karaj, Iran

2 Department of Nuclear Engineering, Science and Research Branch, Islamic Azad University, Tehran, Iran

Abstract

In this experimental work, Polycarbonate/Bismuth Oxide (PC-Bi2O3) nanocomposites were prepared in various concentrations of 0, 10, 30, and 50 wt% with thicknesses of 1 mm and irradiated by a pure beta-emitter source of Sr-90. To fabricate the electrodes, copper sheets with thickness of 100 µm were attached to the top and bottom surfaces of the samples using the silver paste. Then, electric current as the dosimetry response, was measured at various dose rates ranging from 30-102 mSv.h-1 at a fixed voltage of 400 V using an electrometer. Results showed that increasing the Bi2O3 wt% led to improvement in the dosimetry response linearly at various dose rates. Also, the amounts of sensitivities for the samples of 0, 10, 30, and 50 wt% were measured as 20.3, 19.8, 28.6, and 36.7 nC.mSv-1.cm-3, respectively. Regarding the mechanism of beta interaction with a polymer-heavy metal oxide nanocomposite, the Bremsstrahlung radiation can be considered as a dominant effect.

Highlights

  • PC/Bi2O3 nanocomposites at various Bi2O3 weight fractions up to 50 wt% are prepared via the solution method.
  • The samples are exposed to beta rays of Sr-90 at various dose rates ranging from 30 to 102 mSv.h-1.
  • Variation of electric current during the irradiation is measured as the dosimetry response of the samples.
  • Increasing the Bi2O3 wt% leads to improvement in the sensitivity and dosimetry response linearly at various dose rates.

Keywords

Attix, F. H. (2008). Introduction to radiological physics and radiation dosimetry. John Wiley & Sons.
Bohm, J. (1976). A measuring and calibration system for currents down to 10-17 A. Atomkernenergie, 27(2):139-143.
Borg, J. (1996). Dosimetry of low-energy beta radiation. Technical report, Risoe National Lab.
Dozik, Y. V. (2001). Calibration of radiation protection monitoring instruments. Atomnaya Tekhnika za Rubezhom, pages 16-19.
Ehrlich, M., Pruitt, J., and Soares, C. (1985). Standard betaparticle and monoenergetic electron sources for the calibration of beta-radiation protection instrumentation. Final technical report, September 1982-May 1985. Technical report, Nuclear Regulatory Commission, Washington, DC (USA). Div. of Radiation.
Ghergherehchi, M., Afarideh, H., Ghannadi, M., et al. (2010). Proton beam dosimetry: a comparison between a plastic scintillator, ionization chamber and Faraday cup. Journal of Radiation Research, 51(4):423-430.
Hosseini, M., Malekie, S., and Keshavarzi, M. (2021). Analysis of radiation shielding characteristics of magnetite/high density polyethylene nanocomposite at diagnostic level using the MCNPX, XCOM, XMuDat and Auto-Ze programs. Moscow University Physics Bulletin, 76(1):S52-S61.
Hosseini, M. A., Malekie, S., and Kazemi, F. (2022). Experimental evaluation of gamma radiation shielding characteristics of polyvinyl alcohol/tungsten oxide composite: A comparison study of micro and nano sizes of the llers. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment,1026:166214.
Intaniwet, A., Mills, C., Shkunov, M., et al. (2012). Heavy metallic oxide nanoparticles for enhanced sensitivity in semiconducting polymer x-ray detectors. Nanotechnology, 23(23):235502.
ISO-6980-2 (2004). Nuclear energyreference beta particle radiation-Part 2: Calibration fundamentals related to basic quantities characterizing the radiation field.
Kang, H., Min, S., Seo, B., et al. (2020). Low energy beta emitter measurement: A review. Chemosensors, 8(4):106.
Kazemi, F., Malekie, S., et al. (2019). A Monte Carlo study on the shielding properties of a novel polyvinyl alcohol (PVA)/WO3 composite, against gamma rays, using the MCNPX code. Journal of Biomedical Physics & Engineering, 9(4):465.
Knoll, G. F. (2010). Radiation detection and measurement. John Wiley & Sons.
Korostynska, O., Arshak, K., Morris, D., et al. (2007). Radiation-induced changes in the electrical properties of carbon filled PVDF thick _lms. Materials Science and Engineering: B, 141(3):115-120.
L'Annunziata, M. F. (2012). Radiation physics and radionuclide decay. In Handbook of Radioactivity Analysis, pages 1-162. Elsevier.
L'annunziata, M. F. (2016). Radioactivity: introduction and history, from the quantum to quarks. Elsevier.
Malekie, S. and Hajiloo, N. (2017). Comparative study of micro and nano size WO3/E44 epoxy composite as gamma radiation shielding using MCNP and experiment. Chinese Physics Letters, 34(10):108102.
Malekie, S. and Ziaie, F. (2017). A two-dimensional simulation to predict the electrical behavior of carbon nanotube/polymer composites. Journal of Polymer Engineering, 37(2):205-210.
Malekie, S., Ziaie, F., and Esmaeli, A. (2016a). Study on dosimetry characteristics of polymer-CNT nanocomposites: Effect of polymer matrix. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 816:101-105.
Malekie, S., Ziaie, F., Feizi, S., et al. (2016b). Dosimetry characteristics of HDPE-SWCNT nanocomposite for real time application. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 833:127-133.
Malekie, S., Ziaie, F., and Naeini, M. A. (2016c). Simulation of polycarbonate-CNT nanocomposite dosimeter based on electrical characteristics. Kerntechnik, 81(6):647-650.
Mehrara, R., Malekie, S., Kotahi, S. M. S., et al. (2021). Introducing a novel low energy gamma ray shield utilizing Polycarbonate Bismuth Oxide composite. Scientific Reports, 11(1):1-13.
Miramonti, L. (2002). A plastic scintillator detector for beta particles. Radiation Measurements, 35(4):347-354.
Mosayebi, A., Malekie, S., Rahimi, A., et al. (2019). Experimental study on polystyrene-MWCNT nanocomposite as a radiation dosimeter. Radiation Physics and Chemistry,164:108362.
Mosayebi, A., Malekie, S., and Ziaie, F. (2017). A feasibility study of polystyrene/CNT nano-composite as a dosimeter for diagnostic and therapeutic purposes. Journal of Instrumentation, 12(05):P05012.
Quaranta, A., Vomiero, A., and Della Mea, G. (2002). Scintillation mechanism and efficiency of ternary scintillator thin films. IEEE Transactions on Nuclear Science, 49(5):2610-2615.
Rahimi, A., Ziaie, F., Sheikh, N., et al. (2020). Calorimetry system based on Polystyrene/MWCNT nanocomposite for electron beam dosimetry: A new approach. Nanotechnologies in Russia, 15(2):175-181.
Saavedra, M. (2005). Novel organic based nano-composite detector films: The making and testing of cnt doped poly(acrylate) thin films on ceramic chip substrates. Department of Physics, University of Surrey, Guildford, Surrey, 37.
Safdari, S. M., Malekie, S., Kashian, S., et al. (2022). Introducing a novel beta-ray sensor based on polycarbonate/bismuth oxide nanocomposite. Scientific Reports,
12(1):1-10.
Tam, A. K., Boyraz, O., Unangst, J., et al. (2018). Quantumdot doped polymeric scintillation material for radiation detection. Radiation Measurements, 111:27-34.
Torrisi, L. (1997). Radiation damage in polyvinyltoluene (PVT) induced by 50-400 kev helium beams. Radiation Effects and Defects in Solids, 143(1):19-31.
Yanagida, T. (2018). Inorganic scintillating materials and scintillation detectors. Proceedings of the Japan Academy, Series B, 94(2):75-97.